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The increasing demand for high laser powers is placing huge demands on current laser technology. This is now reaching a limit, and to realise new areas of research promised at high intensities, new cost-effective and technically feasible ways of scaling up the laser power and controlling its optical characteristics are required. It is likely that ultra-compact, time-dependent, plasma-based amplifiers and optical elements (such as mirrors, polarisers, waveplates, etc.) will be required to reach powers exceeding tens of petawatts and possibly exawatts, and to manipulate the laser beams. Plasma is a robust optical medium as it is broken-down and can sustain extremely high electric fields. Plasma-based optical elements will most likely require the production of transient plasma gratings (TPGs), which take advantage of the ponderomotive force of the beat of at least two laser pulses. To create an amplifier, the TPG is formed through the action of the beat wave of a pump and seed pulse, which has a phase velocity satisfying the conditions for energy and momentum conservation of the three waves, where the third wave is a Langmuir or ion acoustic wave. Other optical elements will normally require static TPGs produced by degenerate driver pulses. Here we present the results of an experimental campaign conducted at the Central Laser Facility, where we have studied chirped pulse Raman amplification at high intensities. We have used a relatively long duration, frequency chirped, pump pulse to limit the growth of noise amplification, while ensuring amplification of the short seed pulse. We show that by changing the sign of the frequency chirp of the pump, the measured back-scattered and amplified seed energies change significantly. A negative chirp leads to a strong reduction in scattering from thermal density fluctuations, but seed amplification saturates. In contrast, for a positive frequency chirp, scattered energy continues to increase with increasing plasma density, without showing any sign of saturation, for the range of densities studied. From simulations we attribute this observation to the production of a local, long-lived, static TPG that continues to scatter the pump pulse long after it has passed. We will discuss the specific conditions that should be satisfied to produce such a grating. The ability to produce and maintain robust TPGs may provide a breakthrough in technologies for manipulating, reflecting and compressing ultra-intense laser pulses.
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