Asymptotically exact analytical solution of the problem of vibrational quantum beats in molecular electronic transitions

Yuri T. Mazurenko

doi:10.1117/12.146151

17 June 1993 Asymptotically exact analytical solution of the problem of vibrational quantum beats in molecular electronic transitions

Yuri T. Mazurenko

Author Affiliations +

Proceedings Volume 1921, Laser Spectroscopy of Biomolecules; (1993) https://doi.org/10.1117/12.146151
Event: Laser Spectroscopy of Biomolecules: 4th International Conference on Laser Applications in Life Sciences, 1992, Jyvaskyla, Finland

Abstract

In order to calculate the characteristics of vibrational quantum beats we use the Heisenberg (time-domain) approach to the nonlinear properties of vibronic spectra. While using this approach, the intensity of emission may be expressed as the convolution-type integral that contains the nonlinear-response function. To evaluate this integral the Laplace method is applied. In so doing the value of the Stokes shift is used as a natural great parameter. This allowed the simple expressions describing the manifestations of vibrational quantum beats to be obtained.

Citation Download Citation

Yuri T. Mazurenko "Asymptotically exact analytical solution of the problem of vibrational quantum beats in molecular electronic transitions", Proc. SPIE 1921, Laser Spectroscopy of Biomolecules, (17 June 1993); https://doi.org/10.1117/12.146151

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