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Multiple diffraction rings are observed after a pulse laser beam passes through an absorbing dye LB film. The theoretical analysis, based on the model of transverse self-phase modulation, is also given. The saturated nonlinear refractive index n2 is estimated to be 2.0 X 10-8 cm2/W from the number of rings induced in the LB films. The main contribution to this larger nonlinearity is believed to be from laser-induced transformation between H-aggregates and monomers of molecules in the LB films.
Weichong Du,Kangsheng Chen,Yanbin Zhu, andSonghao Liu
"Spatial self-phase modulation in Langmuir-Blodgett films", Proc. SPIE 1979, 1992 International Conference on Lasers and Optoelectronics, (11 May 1993); https://doi.org/10.1117/12.144078
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Weichong Du, Kangsheng Chen, Yanbin Zhu, Songhao Liu, "Spatial self-phase modulation in Langmuir-Blodgett films," Proc. SPIE 1979, 1992 International Conference on Lasers and Optoelectronics, (11 May 1993); https://doi.org/10.1117/12.144078