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Layered two-dimensional (2D) materials possess unique optical properties. For example, the monolayer family of Transition Metal Dichalcogenide (TMD) materials (such as WS2 and MoS2) is well known for the existence of a direct band gap. In this talk, we discuss the characterization of the second order nonlinear susceptibility in mono- or few-layer TMDs, which have been recently shown to exhibit extraordinary second harmonic generation. We investigate the large nonlinear response due to resonance enhancement. Theoretical analysis will be discussed and compared with experimental results.
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Corey Janisch, Ana Laura-Elias, Mauricio Terrones, Zhiwen Liu, "Second order nonlinear characterization of two dimensional materials
(Conference Presentation)," Proc. SPIE 9956, Ultrafast Nonlinear Imaging and Spectroscopy IV, 995609 (2 November 2016); https://doi.org/10.1117/12.2238349