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21 September 2020 Optical studies of semiconductor perovskite nanocrystals for classical optoelectronic applications and quantum information technologies: a review
Zengle Cao, Fengrui Hu, Chunfeng Zhang, Shining N. Zhu, Min Xiao, Xiaoyong Wang
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Abstract

Semiconductor perovskite films are now being widely investigated as light harvesters in solar cells with ever-increasing power conversion efficiencies, which have motivated the fabrication of other optoelectronic devices, such as light-emitting diodes, lasers, and photodetectors. Their superior material and optical properties are shared by the counterpart colloidal nanocrystals (NCs), with the additional advantage of quantum confinement that can yield size-dependent optical emission ranging from the near-UV to near-infrared wavelengths. So far, intensive research efforts have been devoted to the optical characterization of perovskite NC ensembles, revealing not only fundamental exciton relaxation and recombination dynamics but also low-threshold amplified spontaneous emission and novel superfluorescence effects. Meanwhile, the application of single-particle spectroscopy techniques to perovskite NCs has helped to resolve a variety of optical properties for which there are few equivalents in traditional colloidal NCs, mainly including nonblinking photoluminescence, suppressed spectral diffusion, stable exciton fine structures, and coherent single-photon emission. While the main purpose of ensemble optical studies is to guide the smooth development of perovskite NCs in classical optoelectronic applications, the rich observations from single-particle optical studies mark the emergence of a potential platform that can be exploited for quantum information technologies.

CC BY: © The Authors. Published by SPIE under a Creative Commons Attribution 4.0 Unported License. Distribution or reproduction of this work in whole or in part requires full attribution of the original publication, including its DOI.
Zengle Cao, Fengrui Hu, Chunfeng Zhang, Shining N. Zhu, Min Xiao, and Xiaoyong Wang "Optical studies of semiconductor perovskite nanocrystals for classical optoelectronic applications and quantum information technologies: a review," Advanced Photonics 2(5), 054001 (21 September 2020). https://doi.org/10.1117/1.AP.2.5.054001
Received: 12 June 2020; Accepted: 25 August 2020; Published: 21 September 2020
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CITATIONS
Cited by 31 scholarly publications and 1 patent.
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KEYWORDS
Perovskite

Excitons

Absorption

Semiconductors

Optical properties

Nanocrystals

Picosecond phenomena

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